Myron Healey

Character: John Dillinger (archive footage)

Paul Dubov

Character: Alvin Karpis

Sam Edwards

Character: Fred Barker

Richard Crane

Character: Homer Van Meter

Lyle Talbot

Character: Dr. William Guellfe, Plastic Surgeon

Jeanne Carmen

Character: Paula

Tamar Cooper

Character: Bonnie Parker

Baynes Barron

Character: Clyde Barrow

Doug Wilson

Character: Charles Arthur 'Pretty Boy' Floyd

Jim Davis

Character: Police Captain Stewart / Narrator

Sydney Mason

Character: Lieutenant Bill Baxter

Lash LaRue

Character: 'Doc' Barker

Ralph Moody

Character: Arthur 'Pa' Barker

Ann Morriss

Character: Mildred Jaunce - The Lady in Red

Aline Towne

Character: Shirley, Girl with Karpis

Regina Gleason

Character: Hope

Jeanne Bates

Character: Mrs. Ross Baxter

Jean Harvey

Character: 'Ma' Barker (archive footage)

Helen Van Tuyl

Character: Texas Lady Governor (archive footage)